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Visible‐light‐mediated regioselective allylation, benzylation, and silylation of methylene‐malononitriles using allylic/benzylic silane and disilane reagents have been developed, delivering the corresponding allylated, benzylated, and silylated products in moderate to excellent yields. These reactions proceed smoothly with exclusive regioselectivity by employing only an organo‐photoredox catalyst...
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