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Whereas synthetically catalyzed nitrogen reduction (N2R) to produce ammonia is widely studied, catalysis to instead produce hydrazine (N2H4) has received less attention despite its considerable mechanistic interest. Herein, we disclose that irradiation of a tris(phosphine)borane (P3B) Fe catalyst, P3BFe+, significantly alters its product profile to increase N2H4 versus NH3; P3BFe+ is otherwise known...
Whereas synthetically catalyzed nitrogen reduction (N2R) to produce ammonia is widely studied, catalysis to instead produce hydrazine (N2H4) has received less attention despite its considerable mechanistic interest. Herein, we disclose that irradiation of a tris(phosphine)borane (P3B) Fe catalyst, P3BFe+, significantly alters its product profile to increase N2H4 versus NH3; P3BFe+ is otherwise known...
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