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One‐dimensional organic structures with well‐oriented π‐aggregation, strong emission, and ease of processability are desirable for optoelectronic waveguiding devices. Herein, a strategy is developed to attain this objective by self‐assembling platinum(II) acetylides into fluorescent supramolecular polymers via cooperative mechanism. The resulting high‐molecular‐weight supramolecular polymers are capable...
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