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In Tb(Pc)2 single‐molecule magnets, where Pc is phthalocyanine, adsorbed on magnesium oxide, the fluctuations of the terbium magnetic moment are strongly suppressed in contrast to the adsorption on silver. On page 5195, J. Dreiser and co‐workers investigate that the molecules are perfectly organized by self‐assembly, as seen in the scanning tunnelling microscopy image (top part of the design). The...
TbPc2 single‐molecule magnets adsorbed on a magnesium oxide tunnel barrier exhibit record magnetic remanence, record hysteresis opening, perfect out‐of‐plane alignment of the magnetic easy axes, and self‐assembly into a well‐ordered layer.
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