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In addition to the appealing semiconducting properties displayed by layered SnII or PbII halidometallates, intriguing phase‐transition‐induced properties, such as dielectric and ferroelectric properties, have recently been found by us in (benzylammonium)2PbCl4 and (cyclohexylammonium)2PbBr4–4xI4x (x = 0–1). The simple molecular structures of the layered compounds allow further chemical design for...
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