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Tertiary allylic alcohols equipped with a carboxyl group can be smoothly aminated under ambient conditions by a conceptually new and stereoselective protocol under palladium catalysis. The in situ formed Z‐configured γ‐amino acid cyclizes to afford an α,β‐unsaturated γ‐lactam, releasing water as the only byproduct. This practical catalytic transformation highlights the use of a carboxyl group acting...
The first general catalytic and highly stereoselective formation of (Z)‐1,4‐but‐2‐ene diols is described from readily available and modular vinyl‐substituted cyclic carbonate precursors using water as a nucleophilic reagent. These 1,4‐diol scaffolds can be generally prepared in high yields and with ample scope in reaction partners using a simple synthetic method that does not require the presence...
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