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Engineering the surface of the metal clusters with the core structure maintained and tuning their luminescence in a wide range is still a challenge in the nanomaterial research. We modified six mono‐pyridyl ligands with different electronic effects (conjugation effect or induction effect) on a superatomic silver cluster [Ag14(C2B10H10S2)6(CH3CN)8] (denoted as Ag14) through in situ site‐specific surface...
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