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Complex polycyclic compounds resembling some natural alkaloids have been prepared in only three high yielding steps by combining the Ugi or Passerini multicomponent reactions with two metal‐catalyzed cyclizations: an intramolecular Tsuji–Trost reaction of the isocyanide‐derived amide followed by a ring‐closing metathesis. Scaffold diversity may be explored by the appropriate choice of starting unsaturated...
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