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Much effort is devoted to develop agents with superior photoacoustic/photothermal properties for improved disease diagnosis and treatment. Herein, a new fused two isoindigo (DIID)‐based semiconducting conjugated polymer (named PBDT‐DIID) is rationally designed and synthesized with a strong near‐infrared absorption band ranging from 700 to 1000 nm. Water‐dispersing nanoparticles (NPs) of PBDT‐DIID...