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A novel two‐step surface modification method that includes atomic layer deposition (ALD) of TiO2 followed by post‐annealing treatment on spinel LiNi0.5Mn1.5O4 (LNMO) cathode material is developed to optimize the performance. The performance improvement can be attributed to the formation of a TiMn2O4 (TMO)‐like spinel phase resulting from the reaction of TiO2 with the surface LNMO. The Ti incorporation...
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