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Ion migration is a key root‐cause of photocurrent instability in perovskite X‐ray detectors. Although 2D perovskite single crystal (PSC) is a good candidate to suppress ion migration compared with its 3D counterpart, its intrinsic stability still needs to be improved. In this work, it is first envisioned to conquer the ion migration by enhanced chemical bonding; the proposal is further confirmed by...
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