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Nitrogen species distribution during coal pyrolysis with Ca addition in N2, CO2 and Ar was studied at 1000 °C using a horizontal tube furnace. In particular, the effect of Ca on the distribution of nitrogen species in N2 and CO2 atmospheres, which were closer to pyrolysis processes of conversional air and oxy‐fuel combustion in comparison with inert Ar environment, was investigated for the first time...
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