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A stable anode‐free all‐solid‐state battery (AF‐ASSB) with sulfide‐based solid‐electrolyte (SE) (argyrodite Li6PS5Cl) is achieved by tuning wetting of lithium metal on “empty” copper current‐collector. Lithiophilic 1 µm Li2Te is synthesized by exposing the collector to tellurium vapor, followed by in situ Li activation during the first charge. The Li2Te significantly reduces the electrodeposition/electrodissolution...
All‐Solid‐State Batteries
In article number 2206762, Yijie Liu, David Mitlin, and co‐workers report a stable anode‐free all‐solid‐state battery (AF‐ASSB) with a sulfide‐based solid‐electrolyte (argyrodite Li6PS5Cl). The battery is achieved by tuning the wetting of lithium metal on the “empty” copper current‐collector. In the cover image, the sprinting antelope represent the lithium cations rapidly...
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