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Engineering Pt‐free catalysts for hydrogen evolution reaction (HER) with high activity and stability is of great significance in electrochemical hydrogen production. Herein, in situ chemical H intercalation into ultrafine Pd to activate this otherwise HER‐inferior material to form the ultrafine IrPdH hydride as an efficient and stable HER electrocatalyst is proposed. The formation of PdIrH depends...
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