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Introducing the hard second phase into soft matrix and reducing the grain size are key strategies to enhance the strength and wear performance of metallic alloys. Herein, to investigate the effect of hard second phase on the mechanical properties and tribological behavior of face‐centered‐cubic (FCC) CoCrFeNi compositionally complex alloy (CCA), a series of ultrafine‐grained CoCrFeNiWx (x = 0, 0.3,...