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A substrate‐controlled asymmetric total synthesis of (+)‐bermudenynol, a compact and synthetically challenging C15Laurencia metabolite that contains several halogen atoms, is reported. The oxocene core, which contains a vinyl chloride, was constructed by an efficient and highly stereoselective intramolecular amide enolate alkylation (IAEA). This result showcases the broad utility of the IAEA methodology...
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