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The discovery of 2D layered MoSi2N4 and WSi2N4 without knowing their 3D parents by chemical vapor deposition in 2020 has stimulated extensive studies of 2D MA2Z4 system due to its structural complexity and diversity as well as versatile and intriguing properties. Here, a comprehensive overview on the state‐of‐the‐art progress of this 2D MA2Z4 family is presented. Starting by describing the unique...
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