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Selective hydrogenolysis of glycerol to 1,3‐propanediol (1,3‐PDO) is recognized as one of the most promising reactions for the valorization of biomass. Precise activation of C─O bonds of glycerol molecule is the key step to realize the high yield of catalytic conversion. Here, a Pt‐loaded Nb–W composite oxides with crystallographic shear phase for the precise activation and cleavage of secondary C─O...