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2D BiCuSeO is an intrinsic p‐type degenerate semiconductor due to its self‐doping effect, which possesses great potential to fabricate high‐performance 2D–2D tunnel field‐effect transistors (TFETs). However, the controllable synthesis of multinary 2D materials by chemical vapor deposition (CVD) is still a challenge due to the restriction of thermodynamics. Here, the CVD synthesis of quaternary 2D...
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