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Two new non‐centrosymmetric ternary compounds, MgSiAs2 and Mg3Si6As8, are discovered via metal flux and solid‐state synthetic methods. MgSiAs2 belongs to the well‐known II‐IV‐V2 family, which is extensively studied experimentally and computationally for their optical properties. MgSiAs2 is computationally predicted but not experimentally known prior to this work. Mg3Si6As8 crystallizes in a new non‐centrosymmetric...
Loss of the inversion center in the crystal structure is represented by varied bond lengths and distorted bond angles as a tetrahedron passes through a looking glass. In article number 1801589, Kirill Kovnir and co‐workers demonstrate a high tendency for Mg–Si–As compounds to crystallize in non‐centrosymmetric space groups.
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