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Reversible multielectron‐transfer materials are of considerable interest because of the potential impact to advance present electrochemical energy storage technology by boosting energy density. To date, a few oxide‐based materials can reach an electron‐transfer number per metal‐cation (eM) larger than 2 upon a (de)intercalation mechanism. However, these materials suffer from degradation due to irreversible...
Reversible Multielectron‐Transfer Materials
In article number 2202861, Ken Sakaushi, Hiroshi Nishihara, and co‐workers demonstrate a superior multielectron transfer by a two‐dimensional coordination framework based on the abundant elements of C, N and Cu. A unique in‐situ rearrangement of the structure upon the reversible energy storage reaction is the key to the significant electrochemical properties...
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