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A low‐firing SrZnV2O7 ceramic was synthesized via a traditional solid‐state sintering route. The phase formation, grain morphology, and dielectric performance were studied in detail. Rietveld refinements based on XRD data revealed that SrZnV2O7 crystallized in the monoclinic space group P21/n, which was further confirmed by TEM analysis. The dense SrZnV2O7 ceramic with an εr of 11.28, a Qf of 56 660 GHz,...