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The electrochemical reduction of CO2 to hydrocarbons involves a multistep proton‐coupled electron transfer (PCET) reaction. Second coordination sphere engineering is reported to be effective in the PCET process; however, little is known about the actual catalytic active sites under realistic operating conditions. We have designed a defect‐containing metal–organic framework, HKUST‐1, through a facile...
The electrochemical reduction of CO2 to hydrocarbons involves a multistep proton‐coupled electron transfer (PCET) reaction. Second coordination sphere engineering is reported to be effective in the PCET process; however, little is known about the actual catalytic active sites under realistic operating conditions. We have designed a defect‐containing metal–organic framework, HKUST‐1, through a facile...