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Advanced high‐energy‐density sodium‐ion batteries (SIBs) are inseparable from cathode materials with high specific capacities. Layered manganese‐rich oxides (NaxMnO2, 0.6 ≤ x ≤1) are promising cathode materials owing to their ease of intercalation and extraction of a considerable amount of sodium ions. However, lattice interactions, especially electrostatic repulsive forces and anisotropic stresses,...
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