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Heat capacities of the mixed stack organic charge-transfer complex tetrathiafulvalene-p-chloranil have been measured at temperatures between 8 and 300 K. Three kinds of crystal polymorphs are obtained depending on the method of synthesis. One of the two polymorphs obtained by recrystallization from acetonitrile solution exhibits a small heat capacity peak due to the neutral-to-ionic transition (N-I...
The magnetic properties of 4-methacryloylamino-2,2,6,6-tetramethylpiperidine-1-oxyl (MATMP) have been investigated by means of adiabatic heat capacity calorimetry in the 0.08-24 K range. The heat capacities of MATMP showed a magnetic phase transition at 0.15 K and a hump centered around 1 K, arising from the short-range ordering characteristic of low-dimensional magnets. The entropy gain due to...
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