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The velocity and angular distributions of desorbing CO 2 in CO oxidation on Pd(110) were studied under the steady-state conditions with cross-correlation time-of-flight techniques. Sharp changes were found in both distributions at the switching point of the rate-determining step. The velocity curves involved fast and slow components. The fast one, which was suddenly suppressed at the switching...
A Pd(110) surface was exposed to a constant flow of a (NO+CO) mixture. Rates of N 2 , N 2 O, and CO 2 formation were determined over the surface temperature range from 350K to 750K in angular-resolved form in a plane in the [001] direction. N 2 desorption showed a two-directional desorption approximated by cos 28 (θ±41°), while N 2 O followed a simple...
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