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Spinel zinc cobalt oxide (ZnCo2O4) is not considered as a superior catalyst for the electrochemical oxygen evolution reaction (OER), which is the bottleneck reaction in water‐electrolysis. Herein, taking advantage of density functional theory (DFT) calculations, we find that the existence of low‐spin (LS) state cobalt cations hinders the OER activity of spinel zinc cobalt oxide, as the t2g6eg0 configuration...
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