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A new asymmetric capacitor concept is proposed providing high energy storage capacity for only one charging direction. Size‐selective microporous carbons (w<0.9 nm) with narrow pore size distribution are demonstrated to exclusively electrosorb small anions (BF4−) but size‐exclude larger cations (TBA+ or TPA+), while the counter electrode, an ordered mesoporous carbon (w>2 nm), gives access to...
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