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Ether solvents with superior reductive stability promise excellent interphasial stability with high‐capacity anodes while the limited oxidative resistance hinders their high‐voltage operation. Extending the intrinsic electrochemical stability of ether‐based electrolytes to construct stable‐cycling high‐energy‐density lithium‐ion batteries is challenging but rewarding. Herein, the anion‐solvent interactions...
Charge compensation on anionic redox reaction (ARR) has been promising to realize extra capacity beyond transition metal redox in battery cathodes. The practical development of ARR capacity has been hindered by high‐valence oxygen instability, particularly at cathode surfaces. However, the direct probe of surface oxygen behavior has been challenging. Here, the electronic states of surface oxygen are...
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