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Developing low‐cost, high‐performance, and durable photoanodes is essential in solar‐driven photoelectrochemical (PEC) energy conversion. Sb2S3 is a low‐bandgap (≈1.7 eV) n‐type semiconductor with a maximum theoretical solar conversion efficiency of ≈28% for PEC water splitting. However, bulk Sb2S3 exhibits opaque characteristics and suffers from severe photocorrosion, and thus the use of Sb2S3 as...
The redox reaction centers in natural organisms conducting oxygenic photosynthesis are well arranged in a physically separated manner to convert sunlight into chemical energy efficiently. Mimicking natural photosynthesis via precisely constructing oxidative and reductive reaction centers within photocatalysts is ideal for enhancing catalytic performances in artificial photosynthesis. In this study,...
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