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Boron (B)‐doped Nb3Al superconductors are prepared by mechanical alloying and subsequent sintering process in this work. Then, the critical current density (Jc) of Nb3Al with different amounts of B doping is studied. In the results, it is shown that Jc performance of Nb3Al is improved obviously after B doping. The best Jc value obtained in this work is 2.2 × 104 A cm−2 (4.2 K, 5 T) for Nb3(Al0.9B0.1...