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Nonfullerene acceptors with mediate bandgap play a crucial role in ternary devices as the third component, further boosting the performance of organic solar cells (OSCs). Herein, three F‐series acceptors (F‐H, F‐Cl, and F‐2Cl) with mediate bandgap are selected and introduced into the PM6:BDT‐Br binary system as third component to find the detailed influence of end groups with chlorine (Cl) atom substitution...