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First‐principles calculations were employed to study the effects of the addition of ZrO2 on the electrochemical activity and structure of Ir–Zr binary oxide. In the computation model employed, Zr atoms replaced Ir atoms in IrO2 supercells, so as to form a rutile‐type solid solution of Ir1−xZrxO2 (0 ≤ x ≤ 1). IrO2–ZrO2 oxide coatings were prepared on Ti substrates by thermal decomposition. X‐ray diffraction...
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