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Single atomic metal (SAM) doping is reported as an effective strategy to promote the electrochemical property of carbon‐based anode materials for high‐power sodium‐ion batteries (SIBs). However, the effects of SAM with different configurations on solid electrolyte interphase (SEI) and energy storage mechanism of Na+ are not revealed. Herein, Cr single atoms (CrSAs) are reported with controllable configurations...