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Decreasing the Ti3+ defect concentration in SrTiO3 is recognized as the focus of seeking a perfect photocatalytic activity. However, the defect‐engineered SrTiO3 by doping different low‐valence metal ions have no similarly good activity in overall water spitting, of which the reason has not been determined. Here, Na+, K+, and Cs are deliberately doped in SrTiO3 to obtain a close low‐level concentration...
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