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The controllable construction of complex metal–organic coordination polymers (CPs) merits untold scientific and technological potential, yet remains a grand challenge of one‐step construction and modulating simultaneously valence states of metals and topological morphology. Here, a thiocyanuric acid (TCA)‐triggered strategy is presented to one‐step rapid synthesis a double‐crystalline Prussian blue...
LiCoO2 (LCO) cathode materials have attracted significant attention for its potential to provide higher energy density in current Lithium‐ion batteries (LIBs). However, the structure and performance degradation are exacerbated by increasing voltage due to the catastrophic reaction between the applied electrolyte and delithiated LCO. The present study focuses on the construction of physically and chemically...
Sliding‐freestanding triboelectric nanogenerators (SF‐TENGs) are desirable for application in wearable power sources; however, improving their durability is the primary challenge. Meanwhile, few studies focus on enhancing the service life of tribo‐materials, especially from an anti‐friction perspective during dry operation. Herein, for the first time, a surface‐textured film with self‐lubricating...
Low infiltration of cytotoxic T lymphocytes and their exhaustion manifest the two concurrent main hurdles for achieving effective tumor immunotherapy of triple‐negative breast cancer. It is found that Galectin‐9 blockage can revise the exhaustion of effector T cells, meanwhile the repolarization of protumoral M2 tumor‐associated macrophages (TAMs) into tumoricidal M1‐like ones can recruit effector...
Bimetallic nanomaterials (BNMs) have been used in sensing, biomedicine, and environmental remediation, but their multipurpose and comprehensive applications in molecular logic computing and information security protection have received little attention. Herein, This synthesis method is achieved by sequentially adding reactants under ice bath conditions. Interestingly, Ag‐Cr NPs can dynamically selectively...
Discovering new drugs and improving action mechanisms is a promising strategy to overcome chemotherapy ineffectiveness caused by cancer cell apoptosis resistance. Natural products (like cyclic lipopeptides, CLPs) are potential sources of nonapoptotic cell death inducers and can form diverse supramolecular structures, closely relating to their bioactivities. Herein, it is found for the first time that...
Inspired by information exchange and logic functions of life based on molecular recognition and interaction networks, ongoing efforts are directed toward development of molecular or nanosystems for multiplexed chem/biosensing and advanced information processing. However, because of their preparation shortcomings, poor functionality, and limited paradigms, it is still a big challenge to develop advanced...
In article number 1803613, Larysa Baraban, Denys Makarov, and co‐workers present an experimental and theoretical study of visible light‐driven Ag/AgCl Janus micromotors revealing high motility in pure H2O. The propulsion efficiency is dependent on the intensity of visible light and contributed by the coupled effect of the plasmonic light absorption of Ag/AgCl and the efficient photochemical decomposition...
Visible light‐driven nano/micromotors are promising candidates for biomedical and environmental applications. This study demonstrates blue light‐driven Ag/AgCl‐based spherical Janus micromotors, which couple plasmonic light absorption with the photochemical decomposition of AgCl. These micromotors reveal high motility in pure water, i.e., mean squared displacements (MSD) reaching 800 µm2 within 8...
In article number 1802537, Larysa Baraban, Denys Makarov, and co‐workers present novel plasmonic Ag/AgCl‐based spherical Janus micromotors and investigate their collective behavior upon interaction with nonmotile passive beads. An efficient exclusion behavior between Ag/AgCl micromotors and the surrounding passive beads is observed under visible light illumination in pure H2O. The exclusion effect...
Insight is provided into the collective behavior of visible‐light photochemically driven plasmonic Ag/AgCl Janus particles surrounded by passive polystyrene (PS) beads. The active diffusion of single Janus particles and their clusters (small: consisting of two or three Janus particles and large: consisting of more than ten Janus particles), and their interaction with passive PS beads, are analyzed...
Enhanced drug releases in a timely manner during urgent medical treatments would significantly enhance the prognosis of patients. Inspired by the facilitated molecular transports by the potentials, an enhanced drug release strategy driven by mechanical disturbances that widely exist in medical treatment processes is proposed. This strategy is enabled by a functional material comprised of multilayers...
Developing appropriate sulfur cathode materials in carbonate‐based electrolyte is an important research subject for lithium‐sulfur batteries. Although several microporous carbon materials as host for sulfur reveal the effect, methods for producing microporous carbon are neither easy nor well controllable. Moreover, due to the complexity and limitation of microporous carbon in their fabrication process,...
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