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Crystalline carbon nitride (CCN), derived from amorphous polymeric CN, is considered as a new generation of metal‐free photocatalyst because of its high crystallinity. In order to further promote the photocatalytic performance of CCN, p‐type MnO nanoparticles are in situ synthesized and merged with n‐type CCN through a one‐pot process to form p–n heterojunction. The formed interfacial electric field...