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We discuss the design of optimum graphitic microstructures for selective adsorption from gaseous mixtures. Binary mixtures of methane and nitrogen at 293.1 K and pressures up to 1 bar were chosen as model systems. Non-local density functional theory (DFT) was used to predict the adsorption of nitrogen and methane in slit-shaped pores for a pore size range of 0.5-5 nm. Predictions of gas mixture adsorption...
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