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We found that Pt-modified Ir-ReOx/SiO2 acted as an effective catalyst for aqueous phase reforming (APR) and selective C-O hydrogenolysis of glycerol without external hydrogen sources at low temperature of 463K, and that 0.5wt% loaded Ir-ReOx/SiO2 (Pt(0.5)-Ir-ReOx/SiO2) provided 1,2-propanediol (1,2-PrD) and acetol in high total yield of 53% at 81% conversion. The initial activity (TOFinitial) over...
Deoxygenation of sorbitol was carried out over a Pt-modified Ir-ReOx/SiO2 catalyst in biphasic solvent system (n-decane+H2O) without external hydrogen. Good yield of gasoline-ranged products was obtained including C5–C6 alkanes and C2–C6 mono-functionalized compounds such as ketones, alcohols, cyclic ethers and carboxylic acids. The Pt(3wt%)-Ir-ReOx/SiO2 catalyst showed the best performance in the...
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