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The adsorption and decomposition of Fe(CO)5 molecules on a Cu(111) surface were studied using reflection absorption infra-red spectroscopy (RAIRS). At low coverage, at a substrate temperature of 80K, Fe(CO)5 is adsorbed with a D3h structure, in random orientations on Cu(111). For higher coverages at 80K, Fe(CO)5 undergoes a structural rearrangement to a species with C4v symmetry, oriented such that...
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