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The reaction rate of the copper-catalyzed oxidation of iodide by oxygen in an aqueous acidic medium is first order in copper and oxygen concentrations, Michaelis–Menten in pH and a complex, asymmetrical bell shaped function in iodide concentrations. A theoretical, multivariate reaction rate equation was proposed which enabled to optimise the various kinetic coefficients. During the parameter optimisation,...
For the calibration of any model, measurements are necessary. As measurements are expensive, it is of interest to determine beforehand which kind of samples will provide maximal information. Using a criterion related to the Fisher information matrix as a measure for information content, it is possible to design a sampling scheme that will enable the most precise parameter estimates. This approach...
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