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The local coordination environment of central active sites plays a critical role in tuning the catalytic properties of heterogeneous single‐metal‐site catalysts (HSMSCs). However, carbon supports with inert surface properties provide weak interaction with the active sites, which hamper the effective modulation of the coordination structure of HSMSCs. Herein, this work shows that introducing N and...
Novel porous polymers can serve as self‐supporting solid carriers and provide abundant coordination or charged sites for single‐site metals, and thus are emerging as advanced functional materials in heterogeneous catalysis for various transformations traditionally catalyzed by homogeneous systems. A brief overview of the development of this heterogenization given, including the recent advances regarding...
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