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Intermolecular interactions are decisive in controlling optoelectronic properties of molecular materials. Polymorphism in one and the same material gives a unique opportunity to gain a direct insight into the intermolecular contributions. Here, stimulated emission properties in two polymorphs of a dicyanodistyrylbenzene derivative with multiple trifluoromethyl groups in the terminal rings are investigated,...
Three‐in‐one: A novel distyrylbenzene‐based material forms J‐type aggregates in single crystals with highly polarized and bright red emission, giving rise to optical gain narrowing, for which different mechanisms (amplified spontaneous emission, laser emission and stimulated resonance Raman scattering) are observed. These are correlated with the favorable intrinsic and macroscopic properties of the...
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