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Two dioxomolybdenum(VI) complexes, [Mo2O4(HBAP)2L] (1) and [MoO2(HMBI)] (2) (HBAP=((E)-2-(2-hydroxybenzylidene)amino)phenol, HMBI=((E)-N′-(2-hydroxy-3-ethoxybenzylidene)isonicotinohydrazide) and L=(4,4′-dipyridyl)), have been synthesized and structurally characterized by elemental analysis, 1H NMR spectroscopy and X-ray single crystal diffraction analysis. In complex (1), a 1D-chain is formed through...
The synthesis of molecule-based magnets derived from decamethylchromocene, CrCp2∗, and dialkyl dicyanofumarates, DRDCF, R=n-propyl (nPr) and isopropyl (iPr) yields two new members of a family of charge transfer (CT) salts, these being metamagnetic solids isomorphous with and reminiscent of the known diethyl (R=Et) homolog. The antiferromagnetic properties of these compounds contrast sharply with the...
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