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Alpha alumina (α‐Al2O3) are inert materials with outstanding thermal, chemical and mechanical stability. Herein, we fabricate porous single‐crystalline (PSC) α‐Al2O3 monoliths at centimeter scale to endow them with high catalytic activity while maintaining their stability. We reduce PSC α‐Al2O3 monoliths to create oxygen vacancies in lattice and stabilize them by the ordered lattice to construct unsaturated...
Alpha alumina (α‐Al2O3) are inert materials with outstanding thermal, chemical and mechanical stability. Herein, we fabricate porous single‐crystalline (PSC) α‐Al2O3 monoliths at centimeter scale to endow them with high catalytic activity while maintaining their stability. We reduce PSC α‐Al2O3 monoliths to create oxygen vacancies in lattice and stabilize them by the ordered lattice to construct unsaturated...