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Two‐dimensional (2D) organic–inorganic hybrid perovskites, benefiting from their natural anisotropy of quantum‐well motifs and optical properties, have shown remarkable polarization‐dependent responses superior to the 3D counterparts. Here, for the first time, multiwavelength polarization‐sensitive detectors were fabricated by using single crystals of a guanidine‐based 2D hybrid perovskite, (BA)2(GA)Pb...
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