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Formamidinium lead triiodide (FAPbI3) has been demonstrated as the most efficient perovskite system to date, due to its excellent thermal stability and an ideal bandgap approaching the Shockley‐Queisser limit. Whereas, there are intrinsic quantum confinement effects in FAPbI3, which lead to unwanted non‐radiative recombination. Additionally, the black α‐phase of FAPbI3 is unstable under room temperature...
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