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Fresh and used alkali acetate (MOAc with M+=Li+, Na+, K+, Cs+) promoted bimetallic PdAu catalysts were studied to investigate the impact of the alkali metal cations on the deactivation of the catalysts during vinyl acetate (VA) synthesis from ethene and acetic acid. Dynamic reordering of PdAu toward an active Pd1Au1 phase, a less active M2Pd2(OAc)6 and inactive Pd3(OAc)6 complexes determines the overall...
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