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Typical Li‐rich layered oxides are widely regarded as promising cathode candidates for high‐energy‐density Li‐ion batteries because of additional output capacities boosted by oxygen redox activities. However, its commercialized applications are hindered by serious capacity loss and voltage decay related to structural degradation upon cycling. Herein, a Co/Ni‐free biphasic O2/O3‐type layered cathode...
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