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The structural and electronic properties of strontium iodide (SrI2) under hydrostatic and nonhydrostatic compressions up to 20 GPa are investigated using first‐principles calculations. Upon hydrostatic compression, SrI2 undergoes a phase transition from the Pbca structure to a quasilayered Pbcm structure around 13.2 GPa, and the bandgap narrows with increasing pressure. Upon uniaxial compression,...
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